Torsional control by intense pulses.

نویسندگان

  • S Ramakrishna
  • Tamar Seideman
چکیده

We generalize the concepts of alignment and 3D alignment by moderately intense laser pulses to control both the overall rotations and the torsional motions of polyatomic molecules. Torsional control is applied to manipulate charge transfer events, hence introducing a potential route to light controlled molecular switches. Potential applications in areas such as molecular assembly, molecular spectroscopies, energy transfer, and molecule-based junctions are envisioned.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Manipulating the torsion of molecules by strong laser pulses.

We demonstrate that strong laser pulses can induce torsional motion in a molecule consisting of a pair of phenyl rings. A nanosecond laser pulse spatially aligns the carbon-carbon bond axis, connecting the two phenyl rings, allowing a perpendicularly polarized, intense femtosecond pulse to initiate torsional motion accompanied by an overall rotation about the fixed axis. We monitor the induced ...

متن کامل

Numerical Simulation of an Intense Isolated Attosecond Pulse by a Chirped Two-Color Laser Field

We investigate theoretically the high-order harmonic spectrum extension and numerical generation of an intense isolated attosecond pulse from He+ ion irradiated by a two-color laser field. Our simulation results show that the chirp of the fundamental field can control HHG cutoff position. Also, these results show that the envelope forms of two fields are important factors for controlling the re...

متن کامل

Effects of intense laser pulse properties on wake field acceleration in magnetized plasma: Half-Sine Shape (HSS) and Gaussian Shape (GS) pulses

In this paper, we have simulated the excitation of wake fields in the interaction of an intensive laser pulses having Half-Sine and Gaussian time envelopes with a fully ionized cold plasma using particle in cell (PIC) method. We investigated the dependency of wake filed amplitude to different laser and plasma parameters such as laser wavelength, pulse duration and electron number density. In ad...

متن کامل

Dynamics of Atoms & Molecules in Intense Laser Fields

Intense laser fields, comparable in magnitude with the Coulomb field within atoms and molecules, can be generated by focussing high-energy and ultrashort laser pulses. When exposed to such a strongly perturbing field, molecules exhibit various exotic features that cannot be observed in weak laser fields. We are seeking a deeper understanding of the behavior of molecules in intense laser fields,...

متن کامل

Abstract Submitted for the MAR06 Meeting of The American Physical Society Molecular quantum computation by using ultrashort intense laser pulses under the influence of non-Markovian dissipation YUKIYOSHI OHT-

Submitted for the MAR06 Meeting of The American Physical Society Molecular quantum computation by using ultrashort intense laser pulses under the influence of non-Markovian dissipation YUKIYOSHI OHTSUKI, Tohoku University & JST-CREST — We numerically study molecular quantum computation by combining an ensemble of molecular states and shaped ultrashort intense laser pulses through a case study o...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Physical review letters

دوره 99 10  شماره 

صفحات  -

تاریخ انتشار 2007